Author: Karkare, S.S.
Paper Title Page
MOYE6 Spin-Polarized Electron Photoemission and Detection Studies 26
 
  • A.C. Rodriguez Alicea, R. Palai
    University of Puerto Rico, Rio Piedras Campus, San Juan, Puerto Rico
  • O. Chubenko, S.S. Karkare
    Arizona State University, Tempe, USA
  • L. Cultrera
    BNL, Upton, New York, USA
 
  Funding: Brookhaven National Laboratory and the Department of Energy of United States under contract No. DE-SC0012704 Also, the Center for Bright Beams, NSF award PHY-1549132.
The experimental investigation of new photocathode ma- terials is time-consuming, expensive, and difficult to accom- plish. Computational modelling offers fast and inexpensive ways to explore new materials, and operating conditions, that could potentially enhance the efficiency of polarized electron beam photocathodes. We report on Monte-Carlo simulation of electron spin polarization (ESP) and quantum efficiency (QE) of bulk GaAs at 2, 77, and 300 K using the data obtained from Density Functional Theory (DFT) cal- culations at the corresponding temperatures. The simulated results of ESP and QE were compared with reported exper- imental measurements, and showed good agreement at 77 and 300 K.
 
slides icon Slides MOYE6 [6.235 MB]  
DOI • reference for this paper ※ doi:10.18429/JACoW-NAPAC2022-MOYE6  
About • Received ※ 03 August 2022 — Revised ※ 07 August 2022 — Accepted ※ 11 August 2022 — Issue date ※ 04 September 2022
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MOPA50 Integrated Photonics Structure Cathodes for Longitudinally Shaped Bunch Trains 160
 
  • S.J. Coleman, D.T. Abell, C.C. Hall
    RadiaSoft LLC, Boulder, Colorado, USA
  • R. Kapadia
    University of Southern California, Los Angeles, California, USA
  • S.S. Karkare
    Arizona State University, Tempe, USA
  • S.Y. Kim, P. Piot, J.F. Power
    ANL, Lemont, Illinois, USA
 
  Funding: This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of High Energy Physics under Award Number DOE DE-SC0021681
Compact, high-gradient structure wakefield accelerators can operate at improved efficiency using shaped electron beams, such as a high transformer ratio beam shape, to drive the wakes. These shapes have generally come from a photocathode gun followed by a transverse mask to imprint a desired shape on the transverse distribution, and then an emittance exchanger (EEX) to convert that transverse shape into a longitudinal distribution. This process discards some large fraction of the beam, limiting wall-plug efficiency as well as leaving a solid object in the path of the beam. In this paper, we present a proposed method of using integrated photonics structures to control the emission pattern on the cathode surface. This transverse pattern is then converted into a longitudinal pattern at the end of an EEX. This removes the need for the mask, preserving the total charge produced at the cathode surface. We present simulations of an experimental set-up to demonstrate this concept at the Argonne Wakefield Accelerator.
 
DOI • reference for this paper ※ doi:10.18429/JACoW-NAPAC2022-MOPA50  
About • Received ※ 03 August 2022 — Revised ※ 05 August 2022 — Accepted ※ 26 August 2022 — Issue date ※ 03 October 2022
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TUYD3 The Quest for the Perfect Cathode 281
 
  • J.W. Lewellen, J. Smedley, T. Vecchione
    SLAC, Menlo Park, California, USA
  • D. Filippetto
    LBNL, Berkeley, California, USA
  • S.S. Karkare
    Arizona State University, Tempe, USA
  • J.M. Maxson
    Cornell University (CLASSE), Cornell Laboratory for Accelerator-Based Sciences and Education, Ithaca, New York, USA
  • P. Musumeci
    UCLA, Los Angeles, California, USA
 
  Funding: U.S. Department of Energy.
The next generation of free electron lasers will be the first to see the performance of the laser strongly dependent on the materials properties of the photocathode. A new injector proposed for the LCLS-II HE is an example of this revolution, with the goal of increasing the photon energy achievable by LCLS-II to over 20 keV. We must now ask, what is the optimal cathode, temperature, and laser combination to enable this injector? There are many competing requirements. The cathode must be robust enough to operate in a superconducting injector, and must not cause contamination of the injector. It must achieve sufficient charge at high repetition rate, while minimizing the emittance. The wavelength chosen must minimize mean transverse energy while maintaining tolerable levels of multi-photon emission. The cathode must be capable of operating at high (~30 MV/m) gradient, which puts limits on both surface roughness and field emission. This presentation will discuss the trade space for such a cathode/laser combination, and detail a new collaborative program among a variety of institutions to investigate it.
 
slides icon Slides TUYD3 [1.632 MB]  
DOI • reference for this paper ※ doi:10.18429/JACoW-NAPAC2022-TUYD3  
About • Received ※ 02 August 2022 — Revised ※ 04 August 2022 — Accepted ※ 14 August 2022 — Issue date ※ 26 September 2022
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TUYD4 Towards High Brightness from Plasmon-Enhanced Photoemitters 285
 
  • C.M. Pierce, I.V. Bazarov, J.M. Maxson
    Cornell University (CLASSE), Cornell Laboratory for Accelerator-Based Sciences and Education, Ithaca, New York, USA
  • D.B. Durham, D. Filippetto, F. Riminucci
    LBNL, Berkeley, California, USA
  • A.H. Kachwala, S.S. Karkare
    Arizona State University, Tempe, USA
  • A. Minor
    UC Berkeley, Berkeley, California, USA
 
  Funding: This work is supported by DOE BES Contract No. DE-AC02-05CH11231. C.P. acknowledges NSF Award PHY-1549132 (CBB) and the US DOE SCGSR program. DD was supported by NSF Grant No. DMR-1548924 (STROBE).
Plasmonic cathodes, whose nanoscale features may locally enhance optical energy from the driving laser trapped at the vacuum interface, have emerged as a promising technology for improving the brightness of metal cathodes. A six orders of magnitude improvement [1] in the non-linear yield of metals has been experimentally demonstrated through this type of nanopatterning. Further, nanoscale lens structures may focus light below its free-space wavelength offering multiphoton photoemission from a region near 10 times smaller [2] than that achievable in typical photoinjectors. In this proceeding, we report on our efforts to characterize the brightness of two plasmonic cathode concepts: a spiral lens and a nanogroove array. We demonstrate an ability to engineer and fabricate nanoscale patterned cathodes by comparing their optical properties with those computed with a finite difference time domain (FDTD) code. The emittance and nonlinear yield of the cathodes are measured under ultrafast laser irradiation. Finally, prospects of this technology for the control and acceleration of charged particle beams are discussed.
[1] Polyakov, A., et al. (2013). Physical Review Letters, 110(7), 076802.
[2] Durham, D. B., et al. (2019). Physical Review Applied, 12(5), 054057.
 
slides icon Slides TUYD4 [7.160 MB]  
DOI • reference for this paper ※ doi:10.18429/JACoW-NAPAC2022-TUYD4  
About • Received ※ 05 August 2022 — Revised ※ 08 August 2022 — Accepted ※ 11 August 2022 — Issue date ※ 13 September 2022
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TUYD5 Epitaxial Alkali-Antimonide Photocathodes on Lattice-matched Substrates 289
 
  • P. Saha, S.S. Karkare
    Arizona State University, Tempe, USA
  • E. Echeverria, A. Galdi, J.M. Maxson, C.A. Pennington
    Cornell University (CLASSE), Cornell Laboratory for Accelerator-Based Sciences and Education, Ithaca, New York, USA
  • E.J. Montgomery, S. Poddar
    Euclid Beamlabs, Bolingbrook, USA
 
  Alkali-antimonides photocathodes, characterized by high quantum efficiency (QE) and low mean transverse energy (MTE) in the visible range of spectrum, are excellent candidates for electron sources to drive X-ray Free Electron Lasers (XFEL) and Ultrafast Electron Diffraction (UED). A key figure of merit for these applications is the electron beam brightness, which is inversely proportional to MTE. MTE can be limited by nanoscale surface roughness. Recently, we have demonstrated physically and chemically smooth Cs3Sb cathodes on Strontium Titanate (STO) substrates grown via co-deposition technique. Such flat cathodes could result from a more ordered growth. In this paper, we present RHEED data of co-deposited Cs3Sb cathodes on STO. Efforts to achieve epitaxial growth of Cs3Sb on STO are then demonstrated via RHEED. We find that films grown epitaxially on substrates like STO and SiC (previously used to achieve single crystalline Cs3Sb) exhibit QE higher than the polycrystalline Cs3Sb cathodes, by an order of magnitude below photoemission threshold. Given the larger QE, lower laser fluence could be used to extract high charge densities, thereby leading to enhanced beam brightness.  
slides icon Slides TUYD5 [2.088 MB]  
DOI • reference for this paper ※ doi:10.18429/JACoW-NAPAC2022-TUYD5  
About • Received ※ 01 August 2022 — Revised ※ 08 August 2022 — Accepted ※ 10 August 2022 — Issue date ※ 07 September 2022
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TUYD6 Design of a 200 kV DC Cryocooled Photoemission Gun for Photocathode Investigations 292
 
  • G.S. Gevorkyan, T.J. Hanks, A.H. Kachwala, S.S. Karkare, C.J. Knill, C.A. Sarabia Cardenas
    Arizona State University, Tempe, USA
 
  Funding: This work was supported by the U.S. National Science Foundation under Award No. PHY-1549132, the Center for Bright Beams, and the DOE under Grant No. DE-SC0021092.
We present the first results of the commissioning of the 200 kV DC electron gun with a cryogenically cooled cathode at Arizona State University. The gun is specifically designed for studying a wide variety of novel cathode materials including single crystalline and epitaxially grown materials at 30 K temperatures to obtain the lowest possible intrinsic emittance of UED and XFEL applications [1]. We will present the measurements of the cryogenic performance of the gun and the first high voltage commissioning results.
[1] G. S. Gevorkyan et. al., Proc. of NAPAC19 MOPLM16 (2019)
 
slides icon Slides TUYD6 [12.632 MB]  
DOI • reference for this paper ※ doi:10.18429/JACoW-NAPAC2022-TUYD6  
About • Received ※ 03 August 2022 — Revised ※ 09 August 2022 — Accepted ※ 11 August 2022 — Issue date ※ 29 September 2022
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TUPA86 Simulations of Nanoblade Cathode Emissions with Image Charge Trapping for Yield and Brightness Analyses 535
 
  • J.I. Mann, G.E. Lawler, J.B. Rosenzweig, B. Wang
    UCLA, Los Angeles, California, USA
  • T. Arias, J.K. Nangoi
    Cornell University, Ithaca, New York, USA
  • S.S. Karkare
    Arizona State University, Tempe, USA
 
  Funding: National Science Foundation Grant No. PHY-1549132
Laser-induced field emission from nanostructures as a means to create high brightness electron beams has been a continually growing topic of study. Experiments using nanoblade emitters have achieved peak fields upwards of 40 GV/m according to semi-classical analyses, begging further theoretical investigation. A recent paper has provided analytical reductions of the common semi-infinite Jellium system for pulsed incident lasers. We utilize these results to further understand the physics underlying electron rescattering-type emissions. We numerically evaluate this analytical solution to efficiently produce spectra and yield curves. The effect of space-charge trapping at emission may be simply included by directly modifying these spectra. Additionally, we use a self-consistent 1-D time-dependent Schrödinger equation with an image charge potential to study the same system as a more exact, but computationally costly, approach. With these results we may finally investigate the mean transverse energy and beam brightness at the cathode in these extreme regimes.
 
DOI • reference for this paper ※ doi:10.18429/JACoW-NAPAC2022-TUPA86  
About • Received ※ 02 August 2022 — Revised ※ 08 August 2022 — Accepted ※ 10 August 2022 — Issue date ※ 03 September 2022
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WEPA65 On-Chip Photonics Integrated Photocathodes 773
 
  • A.H. Kachwala, O. Chubenko, S.S. Karkare
    Arizona State University, Tempe, USA
  • R. Ahsan
    USC, Los Angeles, California, USA
  • H.U. Chae, R. Kapadia
    University of Southern California, Los Angeles, California, USA
 
  Funding: This work is supported by the NSF Center for Bright Beams under award PHY-1549132, and by the Department of Energy, Office of Science under awards DE-SC0021092, and DE-SC0021213.
Photonics integrated photocathodes can result in advanced electron sources for various accelerator applications. In such photocathodes, light can be directed using waveguides and other photonic components on the substrate underneath a photoemissive film to generate electron emission from specific locations at sub-micron scales and at specific times at 100-femtosecond scales along with triggering novel photoemission mechanisms resulting in brighter electron beams and enabling unprecedented spatio-temporal shaping of the emitted electrons. In this work we have demonstrated photoemission confined in the transverse direction using a nanofabricated Si3N4 waveguide underneath a 40-nm thick cesiated GaAs photoemissive film, thus demonstrating a proof of principle feasibility of such photonics integrated photocathodes. This work paves the way to integrate the advances in the field of photonics and nanofabrication with photocathodes to develop better electron sources.
 
poster icon Poster WEPA65 [0.642 MB]  
DOI • reference for this paper ※ doi:10.18429/JACoW-NAPAC2022-WEPA65  
About • Received ※ 26 July 2022 — Revised ※ 06 August 2022 — Accepted ※ 07 August 2022 — Issue date ※ 10 August 2022
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WEPA66 Near-Threshold Photoemission from Graphene Coated Cu Single Crystals 776
 
  • C.J. Knill, S.S. Karkare
    Arizona State University, Tempe, USA
  • H. Ago, K. Kawahara
    Global Innovation Center, Kyushu University, Kasuga, Fukuoka, Japan
  • E. Batista, N.A. Moody, G.X. Wang, H. Yamaguchi, P. Yang
    LANL, Los Alamos, New Mexico, USA
 
  Funding: This work was supported by the U.S. National Science Foundation under Award PHY-1549132, the Center for Bright Beams, and by the Department of Energy under Grant DE-SC0021092.
The brightness of electron beams emitted from photocathodes plays a key role in the performance of x-ray free electron lasers (XFELs) and ultrafast electron diffraction (UED) experiments. In order to achieve the maximum beam brightness, the electrons need to be emitted from photocathodes with the smallest possible mean transverse energy (MTE). Recent studies have looked at the effect that a graphene coating has on the quantum efficiency (QE) of the cathode [1]. However, there have not yet been any investigations into the effect that a graphene coating has on the MTE. Here we report on MTE and QE measurements of a graphene coated Cu(110) single crystal cathode at room and cryogenic temperatures. At room temperature, a minimum MTE of 25 meV was measured at 295 nm. This MTE remained stable at 25 meV over several days. At 77 K, the minimum MTE of 9 meV was measured at 290 nm. We perform density functional theory (DFT) calculations to look at the effects of a graphene coating on a Cu(111) surface state. These calculations show that the graphene coating reduces the radius of the surface state, allowing for emission from a lower transverse energy state in comparison to bare Cu(111).
[1] F. Liu et al, Appl. Phys. Lett. 110, 041607 (2017); https://doi.org/10.1063/1.4974738
 
DOI • reference for this paper ※ doi:10.18429/JACoW-NAPAC2022-WEPA66  
About • Received ※ 28 July 2022 — Revised ※ 19 July 2022 — Accepted ※ 07 August 2022 — Issue date ※ 10 August 2022
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